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APPLICATION OF COMPUTATIONAL MODELING AND SIMULATIONS FOR UNDERSTANDING MODES OF PHOSPHATIDYLCHOLINE SPECIFIC NATURAL ANTIBODY BINDING
Dissertation

APPLICATION OF COMPUTATIONAL MODELING AND SIMULATIONS FOR UNDERSTANDING MODES OF PHOSPHATIDYLCHOLINE SPECIFIC NATURAL ANTIBODY BINDING

Anna Nancy Fraser-Philbin
Doctor of Philosophy (PHD), Creighton University
2026

Abstract

Antibody cloning B-1 B cells Homology modeling Light chain selection Phosphatidylcholine reactive antibodies Molecular Dynamics
Natural antibodies (nAbs) are immunoglobulins that arise without prior exposureto exogenous antigens, providing immediate defense against pathogens and contributing to tissue homeostasis, clearance of apoptotic cells, and regulation of inflammation. Despite these roles, nAbs remain understudied relative to conventionally adaptive antigen-specific antibodies, partly due to their polyreactivity, low affinity, and complex regulation. Among nAbs, phospholipid-reactive antibodies constitute a key subset recognizing endogenous lipid antigens, including phosphatidylcholine (PtC), an essential phospholipid commonly found in cell membranes. Previous sequencing of PtC-reactive (PtC+) antibodies using the VH12 heavy chain revealed distinct skewing of light chain gene usage. Studying PtC+ nAbs is difficult because their polyreactivity and low affinity makes distinguishing specific binding from artifact difficult in traditional immunoassays. Computational methods offer alternative models. Structural modeling and in silico simulations enable prediction and visualization of antibody-antigen interactions to decipher modes of binding, affinities, and specificity determinants of PtC+ nAbs. Here we present evidence that KV4-91 KJ gene usage skews away from [KJ1] due to not forming an accessible binding site and towards [KJ5] in receptor editing deficient mice because it creates a nAb with a higher binding affinity to PtC. Lastly, we show that antibody-PtC binding is directed towards the phospholipid headgroup. Computational approaches can reveal patterns in antibody repertoires, identify key structural motifs, and guide future experimental validation.
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Fraser-Philbin_A_2026_PhD4.98 MB
Embargoed Access, Embargo ends: 06/01/2027

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